I played around some more with 10.13.5 beta, and I think Centrify working may have just been dumb luck the one time I tried it. While the smartcard unlocked in Keychain Access the first time it was inserted, removing and reinserting it resulted in it not working. Also, running the Centrify diagnostics resulted in 3-4 prompts for my PIN before it completed. Implementing the fix identified earlier in the thread resulted in the smartcard always unlocking even after being removed and reinserted, and running the Centrify diagnostics completed with only one PIN prompt.
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